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Dynamic Solvent System as a novel approach to sustainable MOF crystallization.
Green Chem., 2025, Accepted Manuscript
DOI: 10.1039/D5GC01029B, Paper
Open Access 
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Leonid Shupletsov, Alina Christin Schieck, Irena Senkovska, Volodymyr Bon, Stefan Kaskel
Herein we report a novel and green synthetic approach for pyrazolate-based metal-organic frameworks (MOFs) as demonstrated by the three prominent examples of this material class: [Ni(bdp)]n, and two supramolecular isomers...
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DOI: 10.1039/D5GC01029B, Paper
Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Leonid Shupletsov, Alina Christin Schieck, Irena Senkovska, Volodymyr Bon, Stefan KaskelHerein we report a novel and green synthetic approach for pyrazolate-based metal-organic frameworks (MOFs) as demonstrated by the three prominent examples of this material class: [Ni(bdp)]n, and two supramolecular isomers...
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Trifluoromethanesulfinyl chloride: an effective trifluoromethyl radical source in the trifluoromethylimination of alkenes
DOI: 10.1039/D5GC01651G, CommunicationJiayu Liang, Shuping Wang, Xingda Zhao, Weilong Lin
CF3SOCl as CF3 source to achieve catalyst-free, highly regioselective intermolecular trifluoromethylimination of alkenes towards β-trifluoromethylamines.
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Porous liquids for gas capture and separation: recent progress and future aspects
Green Chem., 2025, Accepted Manuscript
DOI: 10.1039/D5GC03111G, Critical ReviewLisha Sheng, Hailong Ning, Yi Wang, Chengyi Li, Shengtao Huang, Yuquan Zhang, Bo Xu, Zhenqian Chen
Porous liquids are a novel class of porous materials, which integrate the permanent porosity of solids with the fluidity of liquids. By rational combination of the porous solids and liquid...
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DOI: 10.1039/D5GC03111G, Critical ReviewLisha Sheng, Hailong Ning, Yi Wang, Chengyi Li, Shengtao Huang, Yuquan Zhang, Bo Xu, Zhenqian Chen
Porous liquids are a novel class of porous materials, which integrate the permanent porosity of solids with the fluidity of liquids. By rational combination of the porous solids and liquid...
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Organic-electrical reduction of carbon–carbon double bonds
DOI: 10.1039/D5GC01804H, Tutorial ReviewBaojie Wang, Yile Song, Jiaxiu Liu, Ke Li, Lirong Wen, Ming Li, Weisi Guo, Lin-Bao Zhang
Organic electrochemical synthesis has become a practical and environmentally friendly synthesis method and is widely used in oxidation, reduction, and redox-neutral reactions.
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Renewable energy-driven synthesis of bioactive quinolinones through photocatalytic and electrochemical activation
DOI: 10.1039/D5GC02521D, CommunicationQingge Zhao, Mengyu Peng, Huimin Li, Longqiang Zhao, Xinyue Song, Peiyao Zhao, Shoucai Wang, Guangbin Jiang, Fanghua Ji
We developed a dual photocatalytic/electrochemical system enabling sustainable, mild, and oxidant-free synthesis of quinolin-2(1H)-ones with broad scope, directly accessing pharmaceutical derivatives.
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Toughened commercial poly(L-lactide) (PLLA) using degradable and recyclable poly(ester-alt-ether)-b-PLLA
DOI: 10.1039/D5GC02301G, Paper
Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Alexander R. Craze, Ryan. W. F. Kerr, Thomas M. McGuire, Lukas Wille, Charlotte. K. WilliamsProperties of bio-derived poly(L-lactide) are improved by block polymer additives which deliver efficient chemical recycling and enzymatic hydrolysis. Blends compete with poly(acrylonitrile-butadiene-styrene) and high impact polystyrene.
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Innovative bacterial cellulose and UiO-66 composites for superior zinc ion battery separator performance
DOI: 10.1039/D5GC01051A, PaperTian Zhao, Pengcheng Xiao, Saiqun Nie, Jiangrong Yu, Shilin Peng, Jiayao Chen, Fuli Luo, Yi Chen
Pure BC separator lack channels, causing loose Zn2+ deposition and dendrites. In situ UiO-66 growth on BC forms hierarchical pores for uniform Zn2+ diffusion/deposition, suppressing dendrites, improving cycling and reducing energy use and emissions.
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Advancing solar-driven redox processes: pyrene-based covalent organic frameworks for efficient environmental remediation and H2O2 production
DOI: 10.1039/D5GC01711D, PaperA. Yaxuan Zheng, B. Siyu Han, C. Yuxin Sun, D. Zhangpei Chen, E. Yuqiu Huo, F. Jianshe Hu
The rational design of efficient photocatalysts is critical for solar-driven chemical conversions.
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Co-recycling of spent cathode and anode via redox-mediated lithiation
DOI: 10.1039/D5GC02248G, PaperZhimin Du, Peixiang Gao, Yuxiang Chen, Yingming Zhang, Yongzhi Liu, Xuejing Qiu, Lingling Xie
Co-recycling of spent cathode/anode via redox-mediated lithiation enables anodic de-lithiation and cathodic re-lithiation, regenerating Al, Cu, graphite and LiFePO4.
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Catalytic hydrogenolysis of lignin under a syngas atmosphere: the enhancement of Cβ–O bond cleavage with CO
DOI: 10.1039/D5GC01618E, PaperXinjun He, Mengqiao Gao, Fukun Li, Zhiyang Tang, Jie Qu, Jinxing Long, Qiang Zeng, Xuehui Li
A syngas atmosphere is more suitable than a pure hydrogen atmosphere for lignin hydrogenolysis, and higher monomer yields can be achieved under a syngas atmosphere.
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Recent advancements in catalytic CO2 conversion to methanol: strategies, innovations, and future directions
DOI: 10.1039/D5GC01906K, Critical ReviewMuhammad Tahir Khalil, Xianli Wu, Shuling Liu, Yanyan Liu, Saima Ashraf, Ruofan Shen, Huanhuan Zhang, Zhikun Peng, Jianchun Jiang, Baojun Li
The catalytic CO2 to methanol conversion enables sustainable fuel production and emissions reduction. Advanced catalysts, reaction mechanisms, and process optimization are critically analyzed.
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Sustainable synthesis of 1-thiol-3-alkyl bicyclo[1.1.1]pentanes via electron donor–acceptor complex photoactivation: a metal- and additive-free strategy for bioisostere design
DOI: 10.1039/D5GC02067K, PaperRuiyuan Xu, Binye Cao, Yibo Wang, Jingyi Zhang, Yuping Huang, Wanmei Li
This study demonstrates a green multicomponent reaction driven by electron donor–acceptor (EDA) complex photoactivation, enabling direct alkylation and thiolation of [1.1.1]propellane under metal- and additive-free conditions.
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Regulation of lithium ion transport dynamics via a carbonized-polymer-dot-modified substrate to achieve 2 mV ultralow voltage hysteresis
DOI: 10.1039/D5GC02081F, PaperJiayu Zhang, Yanfei Li, Yihan Song, Guoduo Yang, Zhuo Wang, Xinyao Huang, Haizhu Sun
This study explores the correlation between voltage hysteresis and cycling stability in lithium metal batteries, achieving an ultra-low hysteresis of 2 mV through carbonized polymer dots, advancing battery technology.
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Rational design of direct and indirect electron transfer pathways to engineer efficient electroactive Escherichia coli for green bioelectrochemical system applications
DOI: 10.1039/D5GC02722E, PaperJiao Feng, Wenjing Yang, Yao Liu, Yan Zhao, Sheng Xu, Xin Wang, Kequan Chen
An electroactive Escherichia coli is constructed through the reasonable design and interaction of multiple electron transfer pathways and applied in a BES.
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Complementary acid site mechanisms in hydrogen-free polyethylene upcycling: elucidating the distinct roles of Brønsted and Lewis sites in Ce-modified zeolites
DOI: 10.1039/D5GC01799H, PaperTaeeun Kwon, Jonghyun Park, Ki Hyuk Kang, Dae Sung Jung, Wangyun Won, Insoo Ro
Hydrogen-free upcycling of polyolefins over zeolite catalysts yields up to 88.7% naphtha. A linear structure–function relationship reveals that Brønsted acid sites promote β-scission, while strong Lewis acid sites enhance hydride abstraction.
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Photoinduced 1,2-cis glycosidation with catalytic amounts of NIS: minimizing the requirements for donor activation and additive dependent anomeric stereocontrol
DOI: 10.1039/D5GC01243K, PaperJianwu Lv, Yongshun Qiu, Yuanyuan Li, Tianlu Li, Richard R. Schmidt, Peng Peng
We describe a simple and practical protocol utilizing 8% NIS in MTBE for efficient 1,2-cis glycosidations.
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Hierarchical phosphorus-enriched organic polymer supports for immobilized palladium catalysts: enabling green and efficient Buchwald–Hartwig amination
DOI: 10.1039/D5GC02325D, PaperXin Liu, Xinxin Han, Jiaxi Cai, Qiaoya Wang, Le Liu, Xin-Hua Duan, Mingyou Hu
Heterogeneous palladium catalysts supported on phosphorus-rich cross-linked organic polymers provide a sustainable solution to the scarcity of Pd resources in the chemical industry.
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Porphyrin-based metal–organic frameworks anchored with Cu species for highly efficient electrocatalytic CO2 reduction to CH4
DOI: 10.1039/D5GC02085A, PaperWeiqi Cao, Dexin Yang, Bingyu Li, Yulan Mi, Kongsheng Qi, Yidan Mao, Yuhua Zhao, Hongping Li, Zhen-Hong He
The Cu-PMOF showed excellent selectivity for the electroreduction of CO2 to CH4, reaching a peak Faradaic efficiency of 80.4% at −300 mA cm−2 and achieving a maximum partial current density of −337.5 mA cm−2 at −1.23 V versus RHE.
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Developing and improving enzyme-driven technologies to synthesise emerging prebiotics
DOI: 10.1039/D5GC01723H, Tutorial Review
Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Noelia Losada-Garcia, Milica Simović, Marija Ćorović, Ana Milivojević, Nikola Nikačević, Cesar Mateo, Dejan Bezbradica, Jose M. PalomoThis review highlights the enzymatic advances in the synthesis of emerging prebiotics, focusing on improved control, biocatalyst enhancement, and bioprocess intensification.
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Methanol production in a sustainable, mild and competitive process: concept launch and analysis
DOI: 10.1039/D5GC01307K, Paper
Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Phillip Nathrath, Fabian Kroll, David Karmann, Michael Geißelbrecht, Patrick SchühleA novel process for the decentralized production of renewable methanol from wet biomass is presented, operating under mild conditions (<210 °C, <10 bar) with high carbon efficiency and competitive costs.
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